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Defect-induced short-range-order from a spin-ice related state in deformed pyrochlore Co2(OH)3Cl

発表形態:
原著論文
主要業績:
主要業績
単著・共著:
共著
発表年月:
2008年01月
DOI:
会議属性:
指定なし
査読:
有り
リンク情報:

日本語フィールド

著者:
X.G. Zheng, M. Hagihala, T. Kawae, C.N. Xu
題名:
Defect-induced short-range-order from a spin-ice related state in deformed pyrochlore Co2(OH)3Cl
発表情報:
Phys. Rev. B 77, 024418 1-5 (2008). 巻: 77 ページ: 024418 1-5
キーワード:
Deformed pyrochlore, quantum magnetism, shor-range-order
概要:
抄録:
Recently we observed a kagom�-ice-like partial ferromagnetic order with coexisting fluctuation in a deformed pyrochlore structure Co2(OH)3Cl. Here we show that when lattice defects are present the remaining fluctuating spins in this material further freeze at lower temperatures below T< Tg = 4 K after it initially freezes into the partial ferromagnetic order near TC = 10 K. This low-temperature transition is glass-like requiring an extremely slow relaxation process in Co2(OH)3Cl. Enhanced disorder in (Co1-xAlx)2(OH)3Cl leads to a short-range order for the fluctuating spins. This result can be considered as an interesting analogy to the low-temperature anomaly in defect-containing pure and doped water ice, especially in the light of its relevance to the problem of residual entropy in ice-water or spin-ice transition.

英語フィールド

Author:
X.G. Zheng, M. Hagihala, T. Kawae, C.N. Xu
Title:
Defect-induced short-range-order from a spin-ice related state in deformed pyrochlore Co2(OH)3Cl
Announcement information:
Phys. Rev. B 77, 024418 1-5 (2008). Vol: 77 Page: 024418 1-5
Keyword:
Deformed pyrochlore, quantum magnetism, shor-range-order
An abstract:
Recently we observed a kagom�-ice-like partial ferromagnetic order with coexisting fluctuation in a deformed pyrochlore structure Co2(OH)3Cl. Here we show that when lattice defects are present the remaining fluctuating spins in this material further freeze at lower temperatures below T< Tg = 4 K after it initially freezes into the partial ferromagnetic order near TC = 10 K. This low-temperature transition is glass-like requiring an extremely slow relaxation process in Co2(OH)3Cl. Enhanced disorder in (Co1-xAlx)2(OH)3Cl leads to a short-range order for the fluctuating spins. This result can be considered as an interesting analogy to the low-temperature anomaly in defect-containing pure and doped water ice, especially in the light of its relevance to the problem of residual entropy in ice-water or spin-ice transition.


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